The Transit 5BN-3 military satellite failed to reach orbit on the 21st April, 1964 and 2.1 pounds of radioactive plutonium was spread over a wide area.
Ed ~ The satellite re-entred north of Madagascar. Its' 630 terabequerel of plutonium-238 metal was scattered in the atmosphere of the southern hemisphere - traces of plutonium were detected after a few months.
Transit 5BN-3 was a US military satellite, which was to be used to test a new submarine navigation system. Launch of the Thor Able Star rocket, with the Transit 5BN-3 and Transit 5E-4 satellites, was from the Vandenberg Air Force base on the 21st April, 1964 at 18:50 GMT, but the rocket failed to achieve orbit - the ballistic flight burned up in the atmosphere. The 53 kg satellite carried a SNAP 9A RTG power generator; the 2.1 pounds of radioactive plutonium was spread over a wide area. Read more
After the failure of Transit 5BN-3 to achieve orbit, it was decided that operational satellites would be solar powered. Not only was the cost lower, but the need to obtain special approvals to launch each nuclear-powered satellite and the operational and publicity issues in case of a failure to orbit were unacceptable. Read more